Geometry optimization

Fixed cell

We use DFTK and the GeometryOptimization package to find the minimal-energy bond length of the $H_2$ molecule. First we set up an appropriate DFTKCalculator (see AtomsCalculators integration), for which we use the LDA model just like in the Tutorial for silicon in combination with a pseudodojo pseudopotential (see Pseudopotentials).

using DFTK
using PseudoPotentialData

pseudopotentials = PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf")
calc = DFTKCalculator(;
    model_kwargs = (; functionals=LDA(), pseudopotentials),  # model_DFT keyword arguments
    basis_kwargs = (; kgrid=[1, 1, 1], Ecut=10)  # PlaneWaveBasis keyword arguments
)
DFTKCalculator(functionals=Xc(lda_x, lda_c_pw), pseudopotentials=PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf"), Ecut=10, kgrid=[1, 1, 1])

Next we set up an initial hydrogen molecule within a box of vacuum. We use the parameters of the equivalent tutorial from ABINIT and DFTK's AtomsBase integration to setup the hydrogen molecule. We employ a simulation box of 10 bohr times 10 bohr times 10 bohr and a pseudodojo pseudopotential.

using LinearAlgebra
using Unitful
using UnitfulAtomic

r0 = 1.4   # Initial bond length in Bohr
a  = 10.0  # Box size in Bohr

cell_vectors = [[a, 0, 0]u"bohr", [0, a, 0]u"bohr", [0, 0, a]u"bohr"]
h2_crude = periodic_system([:H => [0, 0, 0.]u"bohr",
                            :H => [r0, 0, 0]u"bohr"],
                           cell_vectors)
FlexibleSystem(H₂, periodicity = TTT):
    cell_vectors      : [      10        0        0;
                                0       10        0;
                                0        0       10]u"a₀"

    Atom(H,  [       0,        0,        0]u"a₀")
    Atom(H,  [     1.4,        0,        0]u"a₀")

Finally we call minimize_energy! to start the geometry optimisation. We use verbosity=2 to get some insight into the minimisation. With verbosity=1 only a summarising table would be printed and with verbosity=0 (default) the minimisation would be quiet.

using GeometryOptimization
results = minimize_energy!(h2_crude, calc; tol_forces=2e-6, verbosity=2)
nothing  # hide
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.110708439425                   -0.82   0.80    6.0    3.70s
  2   -1.117206171050       -2.19       -1.88   0.80    1.0    1.75s
  3   -1.117250518004       -4.35       -2.73   0.80    1.0   19.7ms
  4   -1.117251168375       -6.19       -3.56   0.80    1.0   19.8ms
  5   -1.117251188380       -7.70       -4.01   0.80    1.0   47.8ms
  6   -1.117251190109       -8.76       -5.12   0.80    1.0   20.6ms
  7   -1.117251190141      -10.49       -5.94   0.80    1.0   20.9ms
  8   -1.117251190143      -11.78       -6.16   0.80    2.0   30.0ms
  9   -1.117251190143      -13.16       -6.40   0.80    1.0   21.2ms
 10   -1.117251190143      -13.49       -7.23   0.80    1.0   21.9ms
 11   -1.117251190143      -15.35       -7.82   0.80    1.0   23.7ms
 12   -1.117251190143      -14.75       -8.31   0.80    1.0   21.7ms
 13   -1.117251190143      -15.35       -8.82   0.80    1.0   87.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.117251190143                   -9.13   0.80    1.0    3.78s
  2   -1.117251190143   +  -15.35      -10.24   0.80    1.0   19.0ms

    Geometry optimisation convergence (in atomic units)
┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   0 │ -1.117251190143 │           │   0.0269318 │  22.1s │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.117517998026                   -2.46   0.80    1.0   13.5ms
  2   -1.117520586051       -5.59       -3.49   0.80    1.0   19.0ms
  3   -1.117520612985       -7.57       -4.23   0.80    1.0   19.3ms
  4   -1.117520613449       -9.33       -5.14   0.80    1.0   19.5ms
  5   -1.117520613464      -10.81       -5.92   0.80    1.0   19.7ms
  6   -1.117520613465      -12.14       -6.42   0.80    1.0   20.0ms
  7   -1.117520613465      -13.33       -7.39   0.80    1.0   63.0ms
  8   -1.117520613465      -14.75       -8.18   0.80    1.0   21.3ms
  9   -1.117520613465   +  -15.05       -8.98   0.80    1.0   21.3ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118247264594                   -1.69   0.80    1.0   13.5ms
  2   -1.118339043933       -4.04       -2.70   0.80    1.0   33.1ms
  3   -1.118340011112       -6.01       -3.44   0.80    1.0   19.4ms
  4   -1.118340028552       -7.76       -4.36   0.80    1.0   19.4ms
  5   -1.118340029137       -9.23       -5.12   0.80    1.0   19.9ms
  6   -1.118340029164      -10.57       -5.62   0.80    1.0   20.1ms
  7   -1.118340029166      -11.73       -6.68   0.80    1.0   26.1ms
  8   -1.118340029166      -13.55       -7.58   0.80    1.0   21.2ms
  9   -1.118340029166   +  -14.70       -8.12   0.80    1.0   21.3ms
 10   -1.118340029166      -14.57       -8.55   0.80    1.0   24.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118340029166                   -9.05   0.80    1.0   13.6ms
  2   -1.118340029166      -14.33      -10.36   0.80    1.0   18.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118340029166                  -11.04   0.80    1.0   13.5ms
  2   -1.118340029166      -14.37      -11.41   0.80    1.0   19.1ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   1 │ -1.118340029166 │           │  0.00297055 │  3.17s │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118346721507                   -3.09   0.80    1.0   13.3ms
  2   -1.118346864758       -6.84       -4.11   0.80    1.0   25.7ms
  3   -1.118346866235       -8.83       -4.86   0.80    1.0   19.4ms
  4   -1.118346866261      -10.59       -5.78   0.80    1.0   19.4ms
  5   -1.118346866262      -12.08       -6.55   0.80    1.0   25.5ms
  6   -1.118346866262      -13.42       -7.04   0.80    1.0   20.5ms
  7   -1.118346866262      -14.65       -8.13   0.80    1.0   23.2ms
  8   -1.118346866262      -14.81       -8.95   0.80    1.0   20.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118354724004                   -2.61   0.80    1.0   13.5ms
  2   -1.118356087056       -5.87       -3.62   0.80    1.0   18.9ms
  3   -1.118356101131       -7.85       -4.37   0.80    1.0   22.1ms
  4   -1.118356101377       -9.61       -5.29   0.80    1.0   19.6ms
  5   -1.118356101385      -11.10       -6.06   0.80    1.0   22.3ms
  6   -1.118356101386      -12.45       -6.55   0.80    1.0   20.0ms
  7   -1.118356101386      -13.61       -7.65   0.80    1.0   23.2ms
  8   -1.118356101386      -14.61       -8.45   0.80    1.0   20.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356101386                   -9.24   0.80    1.0   13.3ms
  2   -1.118356101386      -14.48       -9.82   0.80    1.0   21.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356101386                  -10.62   0.80    1.0   13.3ms
  2   -1.118356101386      -14.57      -11.46   0.80    1.0   21.6ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   2 │ -1.118356101386 │     -4.79 │  4.47268e-5 │  535ms │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356102848                   -4.94   0.80    1.0   20.2ms
  2   -1.118356102877      -10.54       -5.96   0.80    1.0   18.9ms
  3   -1.118356102877      -12.52       -6.70   0.80    1.0   24.8ms
  4   -1.118356102877      -14.11       -7.62   0.80    1.0   19.5ms
  5   -1.118356102877      -14.88       -8.39   0.80    1.0   19.8ms
  6   -1.118356102877   +  -14.57       -8.89   0.80    1.0   22.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356104771                   -4.40   0.80    1.0   15.9ms
  2   -1.118356105116       -9.46       -5.42   0.80    1.0   18.7ms
  3   -1.118356105120      -11.45       -6.17   0.80    1.0   21.6ms
  4   -1.118356105120      -13.20       -7.09   0.80    1.0   20.1ms
  5   -1.118356105120      -14.75       -7.86   0.80    1.0   20.2ms
  6   -1.118356105120      -14.70       -8.35   0.80    1.0   83.9ms
  7   -1.118356105120   +  -14.29       -9.45   0.80    1.0   20.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356105120                  -10.08   0.80    1.0   13.6ms
  2   -1.118356105120      -14.57      -11.02   0.80    1.0   19.2ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356105120                  -11.67   0.80    1.0   13.4ms
  2   -1.118356105120   +  -13.92      -12.44   0.80    1.0   19.0ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   3 │ -1.118356105120 │     -8.43 │  1.05409e-8 │  1.10s │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

Structure after optimisation (note that the atom has wrapped around)

results.system
FlexibleSystem(H₂, periodicity = TTT):
    cell_vectors      : [      10        0        0;
                                0       10        0;
                                0        0       10]u"a₀"

    Atom(H,  [-0.0431829, -5.71633e-35, 1.36192e-34]u"a₀")
    Atom(H,  [ 1.44318, -1.10463e-34, -1.45975e-34]u"a₀")

Compute final bond length:

rmin = norm(position(results.system[1]) - position(results.system[2]))
println("Optimal bond length: ", rmin)
Optimal bond length: 1.4863658664184176 a₀

Our result (1.486 Bohr) agrees with the equivalent tutorial from ABINIT.

Variable cell

Recent versions of GeometryOptimization support cell optimization as well by passing variablecell=true to minimize_energy!.

For a plane-wave code like DFTK, variable cells pose an additional challenge: changes to the cell's size affect the used plane waves, leading to discontinuities in the energy and stresses. This can cause the geometry optimization to struggle and/or fail to converge.

A practical strategy to overcome this problem is Energy cutoff smearing. As a demonstration let us find the optimal lattice constant of silicon.

Like before we define a calculator, this time with a kinetic_blowup set to use energy cutoff smearing:

calc = DFTKCalculator(;
    model_kwargs = (; functionals=LDA(), pseudopotentials,
                      kinetic_blowup=BlowupCHV()),
    basis_kwargs = (; kgrid=[2, 2, 2], Ecut=10)
)
DFTKCalculator(functionals=Xc(lda_x, lda_c_pw), pseudopotentials=PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf"), Ecut=10, kgrid=[2, 2, 2])

And here is our starting silicon structure:

a = 10.0u"bohr"   # Approximate Silicon lattice constant
cell_vectors = a/2 * [[0, 1, 1], [1, 0, 1], [1, 1, 0]]
initial_silicon = periodic_system([:Si =>  ones(3)/8,
                                   :Si => -ones(3)/8],
                                  cell_vectors;
                                  fractional=true)
FlexibleSystem(Si₂, periodicity = TTT):
    cell_vectors      : [       0        5        5;
                                5        0        5;
                                5        5        0]u"a₀"

    Atom(Si, [    1.25,     1.25,     1.25]u"a₀")
    Atom(Si, [   -1.25,    -1.25,    -1.25]u"a₀")

We now minimize, passing variablecell=true:

using GeometryOptimization
results = minimize_energy!(initial_silicon, calc; variablecell=true,
                           tol_virial=2e-6, verbosity=2)
nothing  # hide
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.335214985695                   -0.80   0.80    7.7    785ms
  2   -8.340938092061       -2.24       -1.69   0.80    1.3    620ms
  3   -8.341205978179       -3.57       -2.80   0.80    3.0   35.2ms
  4   -8.341214235019       -5.08       -3.27   0.80    3.0   37.8ms
  5   -8.341214268061       -7.48       -3.94   0.80    1.3   26.7ms
  6   -8.341214272418       -8.36       -5.08   0.80    2.3   31.8ms
  7   -8.341214272515      -10.01       -5.55   0.80    3.7   38.5ms
  8   -8.341214272518      -11.59       -6.29   0.80    2.7   32.4ms
  9   -8.341214272518      -12.88       -7.25   0.80    3.0   35.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.341214272518                   -8.35   0.80    1.0    629ms
  2   -8.341214272518      -14.45       -9.49   0.80    1.0   26.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.341214272518                   -9.73   0.80    1.0   25.8ms
  2   -8.341214272518   +    -Inf      -10.11   0.80    1.0   30.5ms

                 Geometry optimisation convergence (in atomic units)
┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────────┤
│   0 │ -8.341214272518 │           │ 5.69311e-33 │    0.163458 │    -0.16 │  30.4s │
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.350570611004                   -1.21   0.80    8.7   78.2ms
  2   -8.351863723203       -2.89       -1.88   0.80    1.3   31.6ms
  3   -8.351926648292       -4.20       -2.80   0.80    3.7   44.8ms
  4   -8.351928506508       -5.73       -3.60   0.80    3.7   45.3ms
  5   -8.351928514098       -8.12       -4.51   0.80    2.7   38.0ms
  6   -8.351928514647       -9.26       -5.36   0.80    3.7   66.1ms
  7   -8.351928514658      -10.95       -6.29   0.80    3.3   45.6ms
  8   -8.351928514658      -12.63       -7.47   0.80    3.7   47.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353392798392                   -1.52   0.80    8.3   76.3ms
  2   -8.353730451491       -3.47       -2.21   0.80    1.0   28.2ms
  3   -8.353757393306       -4.57       -2.97   0.80    4.0   46.0ms
  4   -8.353757521326       -6.89       -4.20   0.80    2.3   35.2ms
  5   -8.353757531654       -7.99       -4.91   0.80    3.7   45.7ms
  6   -8.353757531714      -10.23       -5.70   0.80    2.7   41.2ms
  7   -8.353757531717      -11.54       -6.92   0.80    3.0   42.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531717                   -7.95   0.80    1.0   29.2ms
  2   -8.353757531717      -14.15       -8.60   0.80    1.0   28.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531717                   -8.87   0.80    1.0   24.4ms
  2   -8.353757531717   +  -14.75       -9.24   0.80    1.0   32.5ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531717                   -9.51   0.80    1.0   24.7ms
  2   -8.353757531717      -14.75       -9.72   0.80    1.0   27.6ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────────┤
│   1 │ -8.353757531717 │           │             │   0.0156413 │   -0.016 │  6.11s │
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353716973544                   -3.20   0.80    7.7   68.0ms
  2   -8.353759855993       -4.37       -3.87   0.80    1.0   36.8ms
  3   -8.353770534781       -4.97       -3.86   0.80    6.0   61.3ms
  4   -8.353770537136       -8.63       -4.18   0.80    1.0   28.7ms
  5   -8.353770537174      -10.43       -4.52   0.80    2.3   35.7ms
  6   -8.353770537388       -9.67       -5.47   0.80    1.7   38.9ms
  7   -8.353770537395      -11.20       -6.50   0.80    3.3   43.3ms
  8   -8.353770537395      -13.29       -7.43   0.80    3.0   41.3ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353769027753                   -2.00   0.80    8.3   70.2ms
  2   -8.353874403263       -3.98       -2.71   0.80    1.0   28.0ms
  3   -8.353895042477       -4.69       -3.26   0.80    4.3   52.6ms
  4   -8.353895103146       -7.22       -4.03   0.80    2.3   36.3ms
  5   -8.353895110639       -8.13       -4.91   0.80    2.3   38.6ms
  6   -8.353895110771       -9.88       -5.50   0.80    3.3   44.5ms
  7   -8.353895110775      -11.35       -7.21   0.80    1.7   36.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110775                   -7.36   0.80    1.0   24.8ms
  2   -8.353895110775      -13.50       -7.48   0.80    1.0   28.2ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110775                   -8.11   0.80    1.0   24.6ms
  2   -8.353895110775      -14.05       -8.25   0.80    1.0   28.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110775                   -8.73   0.80    1.0   25.1ms
  2   -8.353895110775      -14.75       -8.85   0.80    1.0   28.1ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────────┤
│   2 │ -8.353895110775 │     -3.86 │             │ 0.000646176 │ -0.00065 │  2.71s │
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353781957688                   -3.64   0.80    8.0   69.9ms
  2   -8.353872241507       -4.04       -3.87   0.80    1.0   28.3ms
  3   -8.353895211671       -4.64       -4.07   0.80    6.3   63.3ms
  4   -8.353895212407       -9.13       -4.30   0.80    1.0   27.9ms
  5   -8.353895212404   +  -11.46       -4.79   0.80    1.7   32.0ms
  6   -8.353895212496      -10.03       -5.11   0.80    1.7   31.8ms
  7   -8.353895212518      -10.66       -5.67   0.80    3.0   37.9ms
  8   -8.353895212520      -11.73       -6.05   0.80    2.0   33.6ms
  9   -8.353895212520      -12.75       -6.12   0.80    1.3   30.2ms
 10   -8.353895212520      -12.71       -6.87   0.80    1.3   30.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353807253253                   -3.29   0.80    8.3   71.2ms
  2   -8.353876859175       -4.16       -3.77   0.80    1.0   38.4ms
  3   -8.353895362316       -4.73       -3.88   0.80    6.0   62.7ms
  4   -8.353895362604       -9.54       -4.41   0.80    1.0   28.5ms
  5   -8.353895362663      -10.23       -4.63   0.80    1.3   30.0ms
  6   -8.353895362680      -10.78       -5.18   0.80    1.0   28.8ms
  7   -8.353895362685      -11.27       -6.08   0.80    2.0   34.0ms
  8   -8.353895362686      -12.35       -6.57   0.80    3.7   43.0ms
  9   -8.353895362686      -13.97       -7.82   0.80    2.0   35.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                   -8.54   0.80    1.0   24.5ms
  2   -8.353895362686   +    -Inf       -9.60   0.80    1.0   27.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                   -9.76   0.80    1.0   23.7ms
  2   -8.353895362686   +  -14.75      -10.14   0.80    1.0   34.0ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                  -10.38   0.80    1.0   24.4ms
  2   -8.353895362686      -14.45      -10.63   0.80    1.0   28.2ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────────┤
│   3 │ -8.353895362686 │     -6.60 │ 2.04192e-32 │  1.72451e-6 │  -1.7e-6 │  2.80s │
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────────┘

Structure after optimization

results.system
FlexibleSystem(Si₂, periodicity = TTT):
    cell_vectors      : [-1.09851e-35  5.27783  5.27783;
                          5.27783 -1.01748e-35  5.27783;
                          5.27783  5.27783 -1.01746e-35]u"a₀"

    Atom(Si, [ 1.31946,  1.31946,  1.31946]u"a₀")
    Atom(Si, [-1.31946, -1.31946, -1.31946]u"a₀")

Since here the cell was rescaled but its shape did not change, we directly extract the optimal lattice constant from one of the cell vectors:

using AtomsBase
amin = AtomsBase.cell_vectors(results.system)[1][2]*2
println("Optimal lattice constant: ", amin)
Optimal lattice constant: 10.555662886539647 a₀

Note that while for silicon the positions of the atoms are fixed by symmetry, in general a variable cell optimization will try to optimize both the cell and the positions of the individual atoms.