Geometry optimization

Fixed cell

We use DFTK and the GeometryOptimization package to find the minimal-energy bond length of the $H_2$ molecule. First we set up an appropriate DFTKCalculator (see AtomsCalculators integration), for which we use the LDA model just like in the Tutorial for silicon in combination with a pseudodojo pseudopotential (see Pseudopotentials).

using DFTK
using PseudoPotentialData

pseudopotentials = PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf")
calc = DFTKCalculator(;
    model_kwargs = (; functionals=LDA(), pseudopotentials),  # model_DFT keyword arguments
    basis_kwargs = (; kgrid=[1, 1, 1], Ecut=10)  # PlaneWaveBasis keyword arguments
)
DFTKCalculator(functionals=Xc(lda_x, lda_c_pw), pseudopotentials=PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf"), Ecut=10, kgrid=[1, 1, 1])

Next we set up an initial hydrogen molecule within a box of vacuum. We use the parameters of the equivalent tutorial from ABINIT and DFTK's AtomsBase integration to setup the hydrogen molecule. We employ a simulation box of 10 bohr times 10 bohr times 10 bohr and a pseudodojo pseudopotential.

using LinearAlgebra
using Unitful
using UnitfulAtomic

r0 = 1.4   # Initial bond length in Bohr
a  = 10.0  # Box size in Bohr

cell_vectors = [[a, 0, 0]u"bohr", [0, a, 0]u"bohr", [0, 0, a]u"bohr"]
h2_crude = periodic_system([:H => [0, 0, 0.]u"bohr",
                            :H => [r0, 0, 0]u"bohr"],
                           cell_vectors)
FlexibleSystem(H₂, periodicity = TTT):
    cell_vectors      : [      10        0        0;
                                0       10        0;
                                0        0       10]u"a₀"

    Atom(H,  [       0,        0,        0]u"a₀")
    Atom(H,  [     1.4,        0,        0]u"a₀")

Finally we call minimize_energy! to start the geometry optimisation. We use verbosity=2 to get some insight into the minimisation. With verbosity=1 only a summarising table would be printed and with verbosity=0 (default) the minimisation would be quiet.

using GeometryOptimization
results = minimize_energy!(h2_crude, calc; tol_forces=2e-6, verbosity=2)
nothing  # hide
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.110529983146                   -0.83   0.80    7.0    5.41s
  2   -1.117182573581       -2.18       -1.87   0.80    1.0    2.33s
  3   -1.117250113827       -4.17       -2.64   0.80    1.0   19.6ms
  4   -1.117251120246       -6.00       -3.43   0.80    1.0   69.7ms
  5   -1.117251188659       -7.16       -4.44   0.80    1.0   19.9ms
  6   -1.117251190128       -8.83       -5.10   0.80    2.0   21.8ms
  7   -1.117251190142      -10.84       -5.77   0.80    1.0   31.7ms
  8   -1.117251190143      -11.96       -6.67   0.80    1.0   20.9ms
  9   -1.117251190143      -13.64       -7.17   0.80    1.0   20.9ms
 10   -1.117251190143      -15.35       -7.75   0.80    1.0   23.3ms
 11   -1.117251190143   +  -14.95       -8.46   0.80    2.0   22.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.117251190143                   -8.94   0.80    1.0    4.28s
  2   -1.117251190143      -14.75      -10.06   0.80    1.0   18.8ms

    Geometry optimisation convergence (in atomic units)
┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   0 │ -1.117251190143 │           │   0.0269318 │  23.5s │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.117517997729                   -2.46   0.80    1.0   72.0ms
  2   -1.117520586046       -5.59       -3.49   0.80    1.0   19.0ms
  3   -1.117520612986       -7.57       -4.23   0.80    1.0   19.2ms
  4   -1.117520613449       -9.33       -5.14   0.80    1.0   19.3ms
  5   -1.117520613465      -10.81       -5.92   0.80    1.0   37.9ms
  6   -1.117520613465      -12.15       -6.43   0.80    1.0   20.3ms
  7   -1.117520613465      -13.37       -7.41   0.80    1.0   20.6ms
  8   -1.117520613465      -15.05       -8.24   0.80    1.0   21.1ms
  9   -1.117520613465      -15.35       -8.93   0.80    1.0   23.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118247264597                   -1.69   0.80    1.0   13.3ms
  2   -1.118339043931       -4.04       -2.70   0.80    1.0   24.6ms
  3   -1.118340011110       -6.01       -3.44   0.80    1.0   18.8ms
  4   -1.118340028551       -7.76       -4.36   0.80    1.0   19.1ms
  5   -1.118340029135       -9.23       -5.12   0.80    1.0   24.7ms
  6   -1.118340029162      -10.57       -5.62   0.80    1.0   19.8ms
  7   -1.118340029164      -11.73       -6.68   0.80    1.0   84.9ms
  8   -1.118340029164      -13.53       -7.58   0.80    1.0   20.7ms
  9   -1.118340029164   +  -14.95       -8.12   0.80    1.0    534ms
 10   -1.118340029164   +  -15.65       -8.55   0.80    1.0   21.2ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118340029164                   -9.05   0.80    1.0   13.1ms
  2   -1.118340029164   +  -14.75      -10.36   0.80    1.0   18.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118340029164                  -11.05   0.80    1.0   13.2ms
  2   -1.118340029164   +  -14.75      -11.42   0.80    1.0   18.4ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   1 │ -1.118340029164 │           │  0.00297055 │  3.63s │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118346721506                   -3.09   0.80    1.0   13.0ms
  2   -1.118346864757       -6.84       -4.11   0.80    1.0   18.5ms
  3   -1.118346866234       -8.83       -4.86   0.80    1.0   18.8ms
  4   -1.118346866260      -10.59       -5.78   0.80    1.0   19.0ms
  5   -1.118346866261      -12.09       -6.55   0.80    1.0   19.4ms
  6   -1.118346866261      -13.40       -7.04   0.80    1.0   19.6ms
  7   -1.118346866261      -15.18       -8.13   0.80    1.0   24.5ms
  8   -1.118346866261      -14.95       -8.95   0.80    1.0   33.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118354724004                   -2.61   0.80    1.0   13.1ms
  2   -1.118356087056       -5.87       -3.62   0.80    1.0   18.4ms
  3   -1.118356101131       -7.85       -4.37   0.80    1.0   18.7ms
  4   -1.118356101377       -9.61       -5.29   0.80    1.0   18.9ms
  5   -1.118356101385      -11.10       -6.06   0.80    1.0   19.4ms
  6   -1.118356101386      -12.45       -6.55   0.80    1.0   19.8ms
  7   -1.118356101386      -13.60       -7.65   0.80    1.0   26.6ms
  8   -1.118356101386      -15.05       -8.45   0.80    1.0   20.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356101386                   -9.24   0.80    1.0   13.0ms
  2   -1.118356101386      -14.21       -9.82   0.80    1.0   18.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356101386                  -10.62   0.80    1.0   13.1ms
  2   -1.118356101386   +  -15.65      -11.46   0.80    1.0   18.4ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   2 │ -1.118356101386 │     -4.79 │  4.47268e-5 │  528ms │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356102848                   -4.94   0.80    1.0   13.3ms
  2   -1.118356102877      -10.54       -5.96   0.80    1.0   18.7ms
  3   -1.118356102877      -12.52       -6.70   0.80    1.0   25.9ms
  4   -1.118356102877      -14.26       -7.62   0.80    1.0   19.1ms
  5   -1.118356102877      -14.70       -8.39   0.80    1.0   19.5ms
  6   -1.118356102877      -14.95       -8.89   0.80    1.0   25.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356104771                   -4.40   0.80    1.0   13.2ms
  2   -1.118356105116       -9.46       -5.42   0.80    1.0   18.4ms
  3   -1.118356105120      -11.45       -6.17   0.80    1.0   21.4ms
  4   -1.118356105120      -13.20       -7.09   0.80    1.0   18.9ms
  5   -1.118356105120      -14.95       -7.86   0.80    1.0   19.5ms
  6   -1.118356105120   +  -14.24       -8.35   0.80    1.0   22.5ms
  7   -1.118356105120      -14.18       -9.45   0.80    1.0   20.2ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356105120                  -10.08   0.80    1.0   13.2ms
  2   -1.118356105120   +  -14.54      -11.02   0.80    1.0   21.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -1.118356105120                  -11.67   0.80    1.0   13.1ms
  2   -1.118356105120      -14.81      -12.44   0.80    1.0   21.6ms

┌─────┬─────────────────┬───────────┬─────────────┬────────┐
│   n │          Energy │ log10(ΔE) │  max(Force) │  Δtime │
├─────┼─────────────────┼───────────┼─────────────┼────────┤
│   3 │ -1.118356105120 │     -8.43 │  9.96223e-9 │  476ms │
└─────┴─────────────────┴───────────┴─────────────┴────────┘

Structure after optimisation (note that the atom has wrapped around)

results.system
FlexibleSystem(H₂, periodicity = TTT):
    cell_vectors      : [      10        0        0;
                                0       10        0;
                                0        0       10]u"a₀"

    Atom(H,  [-0.0431829, -3.0507e-18, 1.37924e-17]u"a₀")
    Atom(H,  [ 1.44318, -1.39711e-17, 1.08881e-17]u"a₀")

Compute final bond length:

rmin = norm(position(results.system[1]) - position(results.system[2]))
println("Optimal bond length: ", rmin)
Optimal bond length: 1.4863658687038097 a₀

Our result (1.486 Bohr) agrees with the equivalent tutorial from ABINIT.

Variable cell

Recent versions of GeometryOptimization support cell optimization as well by passing variablecell=true to minimize_energy!.

For a plane-wave code like DFTK, variable cells pose an additional challenge: changes to the cell's size affect the used plane waves, leading to discontinuities in the energy and stresses. This can cause the geometry optimization to struggle and/or fail to converge.

A practical strategy to overcome this problem is Energy cutoff smearing. As a demonstration let us find the optimal lattice constant of silicon.

Like before we define a calculator, this time with a kinetic_blowup set to use energy cutoff smearing:

calc = DFTKCalculator(;
    model_kwargs = (; functionals=LDA(), pseudopotentials,
                      kinetic_blowup=BlowupCHV()),
    basis_kwargs = (; kgrid=[2, 2, 2], Ecut=10)
)
DFTKCalculator(functionals=Xc(lda_x, lda_c_pw), pseudopotentials=PseudoFamily("dojo.nc.sr.pbe.v0_4_1.standard.upf"), Ecut=10, kgrid=[2, 2, 2])

And here is our starting silicon structure:

a = 10.0u"bohr"   # Approximate Silicon lattice constant
cell_vectors = a/2 * [[0, 1, 1], [1, 0, 1], [1, 1, 0]]
initial_silicon = periodic_system([:Si =>  ones(3)/8,
                                   :Si => -ones(3)/8],
                                  cell_vectors;
                                  fractional=true)
FlexibleSystem(Si₂, periodicity = TTT):
    cell_vectors      : [       0        5        5;
                                5        0        5;
                                5        5        0]u"a₀"

    Atom(Si, [    1.25,     1.25,     1.25]u"a₀")
    Atom(Si, [   -1.25,    -1.25,    -1.25]u"a₀")

We now minimize, passing variablecell=true:

using GeometryOptimization
results = minimize_energy!(initial_silicon, calc; variablecell=true,
                           tol_virial=2e-6, verbosity=2)
nothing  # hide
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.335338117619                   -0.80   0.80    7.3    777ms
  2   -8.340978673747       -2.25       -1.70   0.80    1.3    628ms
  3   -8.341208638636       -3.64       -2.76   0.80    3.0   33.5ms
  4   -8.341214247518       -5.25       -3.33   0.80    3.3   37.8ms
  5   -8.341214270311       -7.64       -4.19   0.80    1.3   26.9ms
  6   -8.341214272490       -8.66       -5.32   0.80    2.7   52.1ms
  7   -8.341214272517      -10.57       -5.68   0.80    3.7   40.2ms
  8   -8.341214272518      -11.99       -7.18   0.80    2.0   29.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.341214272518                   -7.60   0.80    1.0    628ms
  2   -8.341214272518      -14.45       -7.85   0.80    1.0   24.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.341214272518                   -8.53   0.80    1.0   22.0ms
  2   -8.341214272518      -14.75       -8.67   0.80    1.0   24.6ms

              Geometry optimisation convergence (in atomic units)
┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │   ⋯
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────
│   0 │ -8.341214272518 │           │  3.6575e-15 │    0.163458 │    -0.16 │   ⋯
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────
                                                                1 column omitted

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.350579107714                   -1.21   0.80    8.7   68.6ms
  2   -8.351864372241       -2.89       -1.88   0.80    1.3   26.3ms
  3   -8.351926541015       -4.21       -2.80   0.80    3.0   72.3ms
  4   -8.351928504697       -5.71       -3.58   0.80    3.7   40.8ms
  5   -8.351928513903       -8.04       -4.47   0.80    2.7   33.8ms
  6   -8.351928514713       -9.09       -5.49   0.80    3.3   38.5ms
  7   -8.351928514736      -10.65       -6.30   0.80    4.3   43.4ms
  8   -8.351928514736      -13.37       -7.02   0.80    3.0   35.7ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353386340946                   -1.52   0.80    7.7   59.6ms
  2   -8.353728595818       -3.47       -2.21   0.80    1.0   24.8ms
  3   -8.353757383906       -4.54       -2.98   0.80    3.3   36.9ms
  4   -8.353757521592       -6.86       -4.22   0.80    2.3   49.0ms
  5   -8.353757531640       -8.00       -5.27   0.80    4.7   44.5ms
  6   -8.353757531660      -10.70       -5.88   0.80    3.0   37.1ms
  7   -8.353757531660      -12.10       -7.08   0.80    3.0   35.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531660                   -7.89   0.80    1.0   22.2ms
  2   -8.353757531660      -14.75       -8.46   0.80    1.0   24.8ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531660                   -9.04   0.80    1.0   27.8ms
  2   -8.353757531660   +  -14.75       -9.26   0.80    1.0   24.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353757531660                   -9.65   0.80    1.0   22.2ms
  2   -8.353757531660      -14.75       -9.98   0.80    1.0   24.8ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │   ⋯
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────
│   1 │ -8.353757531660 │           │ 1.00172e-14 │   0.0156413 │   -0.016 │   ⋯
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────
                                                                1 column omitted

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353708351252                   -3.19   0.80    8.3   62.0ms
  2   -8.353758803863       -4.30       -3.87   0.80    1.0   29.4ms
  3   -8.353770532083       -4.93       -3.80   0.80    6.0   54.3ms
  4   -8.353770536504       -8.35       -4.11   0.80    1.0   25.3ms
  5   -8.353770536906       -9.40       -4.43   0.80    2.0   30.2ms
  6   -8.353770537313       -9.39       -5.05   0.80    1.7   31.4ms
  7   -8.353770537341      -10.56       -5.51   0.80    2.7   33.5ms
  8   -8.353770537343      -11.62       -6.91   0.80    2.3   32.6ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353730803712                   -2.00   0.80    8.7   62.6ms
  2   -8.353870463865       -3.85       -2.72   0.80    1.0   24.8ms
  3   -8.353895051506       -4.61       -3.33   0.80    4.7   44.0ms
  4   -8.353895106071       -7.26       -4.16   0.80    2.3   36.5ms
  5   -8.353895110677       -8.34       -4.90   0.80    3.0   36.8ms
  6   -8.353895110768      -10.04       -5.92   0.80    3.3   38.8ms
  7   -8.353895110771      -11.61       -6.99   0.80    4.0   42.1ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110771                   -7.82   0.80    1.0   22.1ms
  2   -8.353895110771      -14.75       -8.61   0.80    1.0   24.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110771                   -9.04   0.80    1.0   22.4ms
  2   -8.353895110771   +    -Inf       -9.46   0.80    1.0   24.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895110771                   -9.59   0.80    1.0   27.3ms
  2   -8.353895110771      -14.75      -10.04   0.80    1.0   25.0ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │   ⋯
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────
│   2 │ -8.353895110771 │     -3.86 │ 7.87599e-15 │  0.00064618 │ -0.00065 │   ⋯
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────
                                                                1 column omitted

n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353805527313                   -3.53   0.80    7.7   59.6ms
  2   -8.353875230603       -4.16       -3.77   0.80    1.0   30.1ms
  3   -8.353895212065       -4.70       -3.85   0.80    6.7   56.2ms
  4   -8.353895212408       -9.46       -4.05   0.80    1.0   24.9ms
  5   -8.353895212436      -10.56       -4.36   0.80    1.3   26.5ms
  6   -8.353895212496      -10.22       -4.66   0.80    2.0   32.0ms
  7   -8.353895212513      -10.77       -5.07   0.80    1.0   25.8ms
  8   -8.353895212516      -11.44       -5.70   0.80    1.7   28.5ms
  9   -8.353895212517      -12.31       -6.16   0.80    2.3   35.1ms
 10   -8.353895212517      -13.52       -6.44   0.80    1.7   29.3ms
 11   -8.353895212517   +  -14.45       -6.42   0.80    1.3   29.8ms
 12   -8.353895212517      -14.27       -7.52   0.80    1.0   26.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353753728599                   -3.21   0.80    8.0   60.8ms
  2   -8.353862532770       -3.96       -3.37   0.80    1.0   25.1ms
  3   -8.353895355307       -4.48       -3.82   0.80    6.0   57.0ms
  4   -8.353895361041       -8.24       -4.23   0.80    1.3   27.6ms
  5   -8.353895362620       -8.80       -5.30   0.80    2.0   30.1ms
  6   -8.353895362685      -10.19       -5.98   0.80    4.0   41.5ms
  7   -8.353895362685   +  -13.47       -6.12   0.80    2.7   38.1ms
  8   -8.353895362686      -12.49       -7.11   0.80    2.0   31.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                   -7.70   0.80    1.0   22.0ms
  2   -8.353895362686      -14.75       -8.39   0.80    1.0   29.4ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                   -8.98   0.80    1.0   22.3ms
  2   -8.353895362686      -14.45       -9.14   0.80    1.0   24.9ms
n     Energy            log10(ΔE)   log10(Δρ)   α      Diag   Δtime 
---   ---------------   ---------   ---------   ----   ----   ------
  1   -8.353895362686                   -9.57   0.80    1.0   22.1ms
  2   -8.353895362686   +  -14.45       -9.71   0.80    1.0   25.1ms

┌─────┬─────────────────┬───────────┬─────────────┬─────────────┬──────────┬────
│   n │          Energy │ log10(ΔE) │  max(Force) │ max(Virial) │ Pressure │   ⋯
├─────┼─────────────────┼───────────┼─────────────┼─────────────┼──────────┼────
│   3 │ -8.353895362686 │     -6.60 │ 5.65068e-15 │  1.71948e-6 │  -1.7e-6 │   ⋯
└─────┴─────────────────┴───────────┴─────────────┴─────────────┴──────────┴────
                                                                1 column omitted

Structure after optimization

results.system
FlexibleSystem(Si₂, periodicity = TTT):
    cell_vectors      : [-3.05112e-18  5.27783  5.27783;
                          5.27783 -3.05112e-18  5.27783;
                          5.27783  5.27783 -3.05112e-18]u"a₀"

    Atom(Si, [ 1.31946,  1.31946,  1.31946]u"a₀")
    Atom(Si, [-1.31946, -1.31946, -1.31946]u"a₀")

Since here the cell was rescaled but its shape did not change, we directly extract the optimal lattice constant from one of the cell vectors:

using AtomsBase
amin = AtomsBase.cell_vectors(results.system)[1][2]*2
println("Optimal lattice constant: ", amin)
Optimal lattice constant: 10.555662909056702 a₀

Note that while for silicon the positions of the atoms are fixed by symmetry, in general a variable cell optimization will try to optimize both the cell and the positions of the individual atoms.